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- W2057459441 abstract "Abstract A growth kinetic model has been developed from a rigorous thermodynamic perspective to describe the crystal growth rates of NH 4 Cl on the basis of the difference of chemical potentials of NH 4 Cl at solid–liquid interface in aqueous NH 4 Cl, NH 4 Cl‐NaCl, and NH 4 Cl‐MgCl 2 solutions. The solid–liquid equilibrium and activity coefficient of NH 4 Cl are calculated by the newly developed accurate Pitzer model with aid of Aspen Plus™ platform. The predictions of the resulting model are in good agreement with the experimental data published in literature and determined in this work at 283.15–333.15 K within the supersaturation up to 0.1. The kinetic model was subsequently used to analyze the effect of several operation variables, including temperature (283.15–333.15 K), supersaturation (up to 0.1), and NaCl or MgCl 2 concentration (0∼2.5 mol kg −1 ), on the crystal growth rate of NH 4 Cl. The crystal growth rate of NH 4 Cl, with activation energy of 39 kJ mol −1 , is strongly temperature‐dependent and increases with increasing temperature in the three systems investigated. The advantage of MgCl 2 over NaCl on the recovery of NH 4 Cl is theoretically and experimentally illustrated from the thermodynamic and kinetic perspectives with the aid of the established model. © 2011 American Institute of Chemical Engineers AIChE J, 2012" @default.
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- W2057459441 date "2011-03-28" @default.
- W2057459441 modified "2023-10-12" @default.
- W2057459441 title "Kinetic analysis for crystal growth rate of NH4Cl in the NaCl-MgCl2-H2O system with a thermodynamic approach" @default.
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- W2057459441 doi "https://doi.org/10.1002/aic.12604" @default.
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