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- W2057571102 abstract "The photodissociation of doubly excited ${mathrm{H}}_{2}$ has been experimentally investigated. Using the pulsed character of the incident synchrotron radiation, the time analysis of the atomic fragment fluorescence Balmer-ensuremath{alpha} (${mathrm{H}}_{mathrm{ensuremath{alpha}}}$) decay was used for identification of the fragments. The measured branching ratios of the H(3l) fragments at a given photon energy contain information about the dynamic behavior of the photodissociation. The states of the first Rydberg series, ${mathit{Q}}_{1}$(2pensuremath{sigma},nlensuremath{lambda}), dissociating into H(1S)+H(n=3) lead almost to H(1S)+H(3S) fragments; the state involved can be identified from the correlation diagram as the (2p${mathrm{ensuremath{sigma}}}_{mathit{u}}$,4d${mathrm{ensuremath{sigma}}}_{mathit{g}}$) configuration. The photodissociating states of the second Rydberg series, ${mathit{Q}}_{2}$(2pensuremath{pi},nlensuremath{lambda}), lead to H(2p)+H(n=3), the H(n=3) fragments being a mixture of H(3S) and H(3D) in a ratio of about 2:1. In order to identify the relevant ${mathit{Q}}_{2}$ state, the energy ordering in the manifold of the molecular states dissociating into ${mathrm{H}}^{mathrm{*}}$(n=2) and ${mathrm{H}}^{mathrm{*}}$(n=3) has been established by calculating the whole dipole-dipole long-range interaction." @default.
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- W2057571102 doi "https://doi.org/10.1103/physreva.52.4622" @default.
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