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- W2057860473 abstract "We have measured the alignment of Hg(6 $^{3}$${mathit{P}}_{1}$) atoms following off-resonant excitation of the Hg 6 $^{1}mathrm{S}_{0}$--6 $^{3}mathrm{P}_{1}$ transition in the presence of Kr. We present a polarization spectrum for both red and blue wings out to detunings beyond 100 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$. This represents a considerable extension to the existing results, which has been made possible by the use of a pump-and-probe excitation scheme. In the experiment a pulsed laser, detuned from the resonance, creates an alignment in the upper state. This is probed by tuning a delayed second laser to a higher transition and monitoring laser-induced fluorescence from the two-step process. The alignment of the asymptotic Hg(6 $^{3}$${mathit{P}}_{1}$) atoms is determined by comparison of the signals obtained for different relative polarizations of the lasers. We discuss the advantages of this method and the relation of the raw data to the polarizations presented. The results are discussed within the context of a simple quasiclassical model of the process." @default.
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- W2057860473 date "1993-04-01" @default.
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- W2057860473 title "Collisional redistribution in Hg-Kr: Polarization spectrum of the redistributed light" @default.
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- W2057860473 doi "https://doi.org/10.1103/physreva.47.3128" @default.
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