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• W2058039712 abstract "We report a phenomenological model to calculate the high-temperature lattice thermal conductivity of filled skutterudite antimonides. The model needs no phonon resonant scattering terms. Instead, we assume that umklapp processes dominate the high-temperature phonon scattering. In order to represent the anharmonicity introduced by the filling atom, we introduce a Gaussian term into the relaxation time of the umklapp process. The developed model agrees remarkably well with the experimental results of REfCo4Sb12 and REfFe4Sb12 (RE = Yb, Ba, and Ca) alloys. To further test the validity of our model, we calculate the lattice thermal conductivity of nanostructured or multi-filled skutterudites. The calculation results are also in good agreement with experiment, increasing our confidence in the developed anharmonicity model." @default.
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• W2058039712 date "2014-10-22" @default.
• W2058039712 modified "2023-09-30" @default.
• W2058039712 title "Lattice thermal conductivity of filled skutterudites: An anharmonicity perspective" @default.
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• W2058039712 doi "https://doi.org/10.1063/1.4898686" @default.
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