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• W2058063098 abstract "The effect of multivalency manganese doping on the defect structure and enhanced electrical resistivity is studied for the high-temperature piezoelectric ($1ensuremath{-}x$)BiScO${}_{3}$--$x$PbTiO${}_{3}$ (BSPT) solid-solution system by means of multifrequency electron paramagnetic resonance spectroscopy combined with conductivity measurements. The results show that manganese is rather incorporated on a scandium than a titanium site as an isovalent substitute (${mathrm{Mn}}_{mathrm{Sc}}^{ifmmodetimeselsetexttimesfi{}}$) instead of acceptor-type centers, such as ${mathrm{Mn}}_{mathrm{Ti}}^{ensuremath{'}}$, ${mathrm{Mn}}_{mathrm{Ti}}^{ensuremath{'}ensuremath{'}}$, or ${mathrm{Mn}}_{mathrm{Sc}}^{ensuremath{'}}$. The enhanced electric resistivity is found being on the one hand due to the trapping of conduction electrons at the manganese functional center sites (${mathrm{Mn}}_{mathrm{Sc}}^{ifmmodetimeselsetexttimesfi{}}+{e}^{ensuremath{'}}{mathrm{Mn}}_{mathrm{Sc}}^{ensuremath{'}}$). On the other hand, through the formation of ${({mathrm{Mn}}_{mathrm{Sc}}^{ensuremath{'}}ensuremath{-}{V}_{mathrm{O}}^{ifmmodebulletelsetextbulletfi{}ifmmodebulletelsetextbulletfi{}})}^{ifmmodebulletelsetextbulletfi{}}$ defect complexes the ionic conductivity is reduced. Concerning the overall mechanism of charge compensation in that material, both kinds of defects mutually compensate." @default.
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• W2058063098 date "2011-08-23" @default.
• W2058063098 modified "2023-10-12" @default.
• W2058063098 title "Manganese-doped<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mo>(</mml:mo><mml:mn>1</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math>BiScO<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>3</mml:mn></mml:msub></mml:math>–<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi>x</mml:mi></mml:math>PbTiO<mml:math xmlns:mml=http://www.w3.org…" @default.
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• W2058063098 doi "https://doi.org/10.1103/physrevb.84.064113" @default.
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