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• W2058168000 abstract "Intermolecular 13C kinetic isotope effects (KIEs) for the Roush allylboration of p-anisaldehyde were determined using a novel approach. The experimental 13C KIEs fit qualitatively with the expected rate-limiting cyclic transition state, but they are far higher than theoretical predictions based on conventional transition state theory. This discrepancy is attributed to a substantial contribution of heavy-atom tunneling to the reaction, and this is supported by multidimensional tunneling calculations that reproduce the observed KIEs." @default.
• W2058168000 created "2016-06-24" @default.
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• W2058168000 date "2012-04-16" @default.
• W2058168000 modified "2023-10-18" @default.
• W2058168000 title "Isotope Effects and Heavy-Atom Tunneling in the Roush Allylboration of Aldehydes" @default.
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• W2058168000 doi "https://doi.org/10.1021/ol300789a" @default.
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