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• W2058419557 abstract "Additional members of the family of high-Tc molecule-based magnets, V[acceptor]2·yCH2Cl2 have been discovered in which the acceptor is a fluorophenyltricyanoethylene. Varying the number and position of the fluorine substitutions around the phenyl ring results in materials with significantly different magnetic ordering temperatures (Tc’s) ranging from 160 to 300 K. Density functional theory calculations were performed on the neutral and anionic forms of the acceptors that reveal modest correlation between Tc and three calculated quantities: the gas-phase electron affinity, the dihedral angle between the phenyl ring and the olefin, and the Mulliken spin densities on the nitrogen atoms. The electrochemistry of the acceptors has also been examined." @default.
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• W2058419557 date "2008-05-23" @default.
• W2058419557 modified "2023-10-17" @default.
• W2058419557 title "Room-Temperature and Near-Room-Temperature Molecule-Based Magnets" @default.
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• W2058419557 doi "https://doi.org/10.1021/ic702359g" @default.
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