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- W2058422022 abstract "Abstract The equilibrium dynamics in aqueous solutions of copper(II)-glycine system have been investigated by measuring the transverse relaxation time of water protons in a wide concentration range. The use of a general method is illustrated to represent the paramagnetic contribution of the multi-site exchange processes involving paramagnetic site(s) to the measured relaxation time of water protons. It has been experimentally verified that the −NH2 ⇌ H2O proton exchange may be the rate determining step in transferring the effect of paramagnetic relaxation to the measured relaxation time of water protons. The rate constants for the G− + H2O ⇌ HG± + OH− and for the G o − + HG± ⇌ H G o ± + G− protonexchanges are determined. It is shown that the rate constants of the CuG2 + G o − k 2 CuG G o + G− and processes could not be determined individually; only their combination of 3k2 + 2k−3 can be given. A suggestion for the mechanism of the ligand exchange is put forward." @default.
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- W2058422022 date "1981-01-01" @default.
- W2058422022 modified "2023-09-27" @default.
- W2058422022 title "Nmr relaxation studies in solution of transition metal complexes. I. Exchange reactions in aqueous solution of copper(II)-glycine system" @default.
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- W2058422022 doi "https://doi.org/10.1016/s0020-1693(00)90094-x" @default.
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