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- W2058452788 abstract "Total synthesis of cephalotaxine (CET), the parent member of a class of structurally unique antileukemia Cephalotaxus alkaloids, was accomplished on the basis of a conceptually novel strategy featuring transannular reductive skeletal rearrangements as the key transformations for the construction of the pentacyclic ring skeleton of CET. The synthetic potential of the designated Clemmensen−Clemo−Prelog−Leonard reductive rearrangement was demonstrated for the first time in a facile synthesis of the benzazepine subunit of CET. A novel endocyclic enamine (cyclopentenone) annulation was discovered and rationalized as an unusual azo-Nazarov-type cyclization." @default.
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- W2058452788 date "2003-07-04" @default.
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- W2058452788 title "A Novel and Efficient Total Synthesis of Cephalotaxine" @default.
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- W2058452788 doi "https://doi.org/10.1021/ol035098b" @default.
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