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- W2058551136 abstract "Photo-physical properties relevant for optical power limiting in the near-visible and visible regions of the spectrum are reported for a series of substituted diarylalkynyl chalcogenophenes (furans, thiophenes, selenophenes, and tellurophenes). The linear ground and excited state absorption as well as the nonlinear (two-photon) absorption were determined at the time-dependent density functional theory level with use of the hybrid exchange-correlation functionals B3LYP and CAM-B3LYP. A selected number of the theoretically studied molecules were synthesized and characterized experimentally with the use of absorption and luminescence spectroscopy. The photo-physical data are compared to the results from optical power limiting measurements performed in THF solution at a wavelength of 532 nm, with a laser pulse length of 5 ns and pulse energies up to 150 µJ. The best compounds in the present investigation display an energy damping by approximately a factor of 10 at a concentration of 0.010 M." @default.
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- W2058551136 date "2009-04-10" @default.
- W2058551136 modified "2023-10-16" @default.
- W2058551136 title "A theoretical and experimental study of non-linear absorption properties of substituted 2,5-di-(phenylethynyl)thiophenes and structurally related compounds" @default.
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- W2058551136 doi "https://doi.org/10.1080/00268970902845289" @default.
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