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• W2058652037 abstract "Overtone vibration-laser double resonance directly measures the relative importance of vibration-to-vibration and vibration-to-translation-and-rotation energy transfer for HF(v=3 and v=4) at room temperature. The fraction of HF(v) molecules relaxing by V–V energy transfer is 0.44±0.05 and 0.16±0.05 for v=3 and v=4, respectively, compared to 0.59±0.10 for v=2. These measurements show that V–T,R energy transfer is the dominant relaxation mechanism for HF(v≥3) and the observed decreased amount of V–V energy transfer for higher initially excited vibrational levels is in good agreement with a chemiluminescence measurement and several theoretical calculations. The data demonstrate that the magnitude of the energy defects for the component pathways primarily determines the energy transfer mechanism for HF(v=2–4)." @default.
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• W2058652037 date "1986-01-01" @default.
• W2058652037 modified "2023-09-23" @default.
• W2058652037 title "A direct determination of the role of vibration-to-vibration energy transfer in HF(<i>v</i>=3,4) self-relaxation" @default.
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• W2058652037 doi "https://doi.org/10.1063/1.450174" @default.
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