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• W2058672897 abstract "At normal conditions 1,4-diazabicyclo[2.2.2]octane hydrobromide [C(6)H(13)N(2)](+.)Br(-) forms centrosymmetric crystals, space group Pm2, NH(+)...N hydrogen-bonded linear polycationic chains with disordered protons in the structure. As in H(2)O ice Ih, the protons in [C(6)H(13)N(2)](+.)Br(-) crystals remain disordered at low temperatures. Above 0.4 GPa the [C(6)H(13)N(2)](+.)Br(-) crystals transform into a new polar NH(+)...Br(-) hydrogen bonded complex, space group Cmc2. It has been crystallized in-situ in a diamond anvil cell and its structure determined by X-rays. The low-pressure triggering of this transformation indicates that it is a possible source of defects in the real structure at normal conditions, where, along with disproportionation defects, they can be responsible for anomalous dielectric properties, including relaxor-like behavior of NH...N hydrogen-bonded compounds." @default.
• W2058672897 created "2016-06-24" @default.
• W2058672897 creator A5038667320 @default.
• W2058672897 creator A5074604908 @default.
• W2058672897 date "2006-04-29" @default.
• W2058672897 modified "2023-09-24" @default.
• W2058672897 title "Pressure Tuning between NH···N Hydrogen-Bonded Ice Analogue and NH···Br Polar dabcoHBr Complexes" @default.
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• W2058672897 doi "https://doi.org/10.1021/jp061234t" @default.
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