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• W2058743432 abstract "Single crystals of the Cd[Cr2]Se4 spinel with Ga admixtures were grown by chemical transport with an aim to study the influence of gallium concentration on the cation distribution and magnetic properties of the Cd–Cr–Ga–Se system. X-ray crystal structure determination showed that, unlike the system Zn– Ga–Cr2Se4 in which gallium could accommodate both tetrahedral and octahedral sites, in the compounds under study the Ga3+ ions were exclusively substituted for the magnetic Cr3+ ions on octahedral sites, while Cd2+ ions were located on tetrahedral sites of the cubic close-packed sublattice formed by the selenium ions. The chemical composition of these compounds can be written as Cd[Cr2−xGax]Se4 (x=0, 0.02, 0.04, 0.06, 0.13). Compared to the parent CdCr2Se4, such a distribution of the cations led to considerably lowered magnetization in saturation states. The ferromagnetic Curie temperature TC was found to decrease from 129 to 120.2 K, as x varied from 0 to 0.06. The high concentration of Ga3+ (x=0.13) caused the paramagnetic Curie–Weiss temperature θC–W to change the sign to a negative. The nature of the magnetic interactions, developing below TN=214 K, appeared to be altered from the ferro-to-antiferromagnetic ordering. Thus, this type of doping strongly limits the extent of ferromagnetizm in the system Cd–Cr–Ga–Se." @default.
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• W2058743432 date "2001-04-01" @default.
• W2058743432 modified "2023-10-18" @default.
• W2058743432 title "Distribution of Metal Ions and Magnetic Properties in Spinel System CdCr2−xGaxSe4" @default.
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• W2058743432 doi "https://doi.org/10.1006/jssc.2000.9053" @default.
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