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- W2058826067 abstract "Multiphoton vibrational excitation of deuterated hydrazoic acid, DN3, by a CO2 laser (I=10 GW/cm2) leads to dissociation forming DN in both X 3Σ− (spin forbidden) and a 1Δ (spin allowed) electronic states. Under collisionless conditions, the nascent DN fragments were probed via laser induced fluorescence, to determine initial product state distributions. The DN(X 3Σ−) molecules are formed predominantly in the symmetric F1 and F3 spin–rotation states with little population (≤6%) in the antisymmetric F2 levels. There is no significant population (<3%) in excited DN(3Σ−) vibrational levels. The distribution of rotational states is Boltzmann‐like, characterized by a rotational ‘‘temperature’’ of about 920 K for the F1, F3 states and 500 K for F2 levels. Doppler profiles showed a large kinetic energy release of about 10 100 cm−1 total in the triplet channel. The DN(1Δ) products are formed preferentially in the symmetric Δ(A’), e‐labeled lambda doublet levels: Δ(A’)/Δ(A‘)=1.44. The DN(1Δ) is formed with no vibr..." @default.
- W2058826067 created "2016-06-24" @default.
- W2058826067 creator A5036290395 @default.
- W2058826067 creator A5044141870 @default.
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- W2058826067 date "1988-08-01" @default.
- W2058826067 modified "2023-09-26" @default.
- W2058826067 title "Energetics and spin‐ and Λ‐doublet selectivity in the infrared multiphoton dissociation DN3→DN(X 3Σ−,a 1Δ)+N2(X 1Σ+g): Experiment" @default.
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- W2058826067 doi "https://doi.org/10.1063/1.455137" @default.
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