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- W2058902401 abstract "Abstract Raman and IR spectra were obtained of molten AlCl3NH3, AlCl3ND3 and AlBr3NH3 in addition to chloroaluminate mixtures of the AlCl3NH3. The main spectral features of the gaseous AlCl3NH3 molecules having a C3v-symmetry are retained in the molten and glassy states. Some additional bands were observed both in the pure liquid and in mixtures with chloroaluminate melts. The spectra indicated that the discussion reaction 2AlCl3NH3 = AlCl−4 + [AlCl2(NH3)2]+ occurs with K ⋍ 3 × 10−3 (mole fraction basis). Frequency shifts found on liquefaction demonstrate that extensive hydrogen bonding takes place between AlCl3NH3 molecules. This observation is supported by the glass-forming nature of AlCl3NH3. The molecule Al2Cl6NH3 seems to exist in binary AlCl3-AlCl3NH3 melts." @default.
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- W2058902401 date "1986-01-01" @default.
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- W2058902401 title "Vibrational spectra and structure of AlCl3NH3 and molten mixtures with MCl-AlCl3 (M = Li, Na, K OR Cs)" @default.
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- W2058902401 doi "https://doi.org/10.1016/s0277-5387(00)84444-7" @default.
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