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- W2058906469 abstract "Multichain aggregates together with individual macromolecules were detected by light scattering in dilute aqueous solutions of chitosan and of its hydrophobic derivatives bearing 4 mol % of n-dodecyl side groups. It was demonstrated that the size of aggregates and their aggregation numbers increase at the introduction of hydrophobic side groups into polymer chains. The key result concerns the effect of the chain length of individual macromolecules on the aggregation behavior. It was shown that for both unmodified and hydrophobically modified (HM) chitosan, the size of aggregates is independent of the length of single chains, which may result from the electrostatic nature of the stabilization of aggregates. At the same time, the number of macromolecules in one aggregate increases significantly with decreasing length of single chains to provide a sufficient number of associating groups to stabilize the aggregate. The analysis of the light scattering data together with TEM results suggests that the aggregates of chitosan and HM chitosan represent spherical hydrogel particles with denser core and looser shell covered with dangling chains." @default.
- W2058906469 created "2016-06-24" @default.
- W2058906469 creator A5066642013 @default.
- W2058906469 creator A5079507051 @default.
- W2058906469 date "2010-11-24" @default.
- W2058906469 modified "2023-10-02" @default.
- W2058906469 title "Multichain Aggregates in Dilute Solutions of Associating Polyelectrolyte Keeping a Constant Size at the Increase in the Chain Length of Individual Macromolecules" @default.
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- W2058906469 doi "https://doi.org/10.1021/bm100990u" @default.
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