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• W2058938863 abstract "A single crystalline methane hydrate (MH) of high-pressure phase II was synthesized in a diamond anvil cell at P≈1.0 GPa and 50 °C through its decomposition line. Its shape is a hexagonal pillar that suggests MH-II is the hexagonal structure. In situ Raman spectra of the C–H stretching vibrations in the guest CH4 molecules present a broad band at 0.94 GPa and separate into two Raman bands at P≈1.3 GPa and room temperature. By considering the Raman intensities and the pressure dependences of their frequencies, we suggest that there exist two or three CH4 molecules in a large cage if five small cages are fully occupied in the MH-II (sH) phase." @default.
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• W2058938863 date "2004-04-01" @default.
• W2058938863 modified "2023-10-11" @default.
• W2058938863 title "Single-crystal growth of the high-pressure phase II of methane hydrate and its Raman scattering study" @default.
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• W2058938863 doi "https://doi.org/10.1016/j.cplett.2004.02.064" @default.
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