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- W2059312069 abstract "We use recent theoretical results on electrons and phonons in technetium and the properties of the entropy Debye temperature θS to perform a new evaluation of the thermodynamic properties of technetium. In particular, we present values for the Gibbs energy, the enthalpy and the entropy from 300 to 4000 K. We present the entropy at 298.15 K, 0S = 33.0(± 0.3) J mol−1 K−1, the entropy of fusion ΔfS = 13.7(± 1) J mol−1K−1, the melting temperature Tf = 2430(± 30) K and the liquid heat capacity CP(1) = 47(± 2) J mol−1 K−1. From experimental phonon dispersion curves we derive the elastic constants c11 = 433 GPa, c12 = c13 = 199 GPa, c44 = 117 GPa and c33 = 470 GPa with an uncertainty of about 3%. These values give the elastic limit Debye temperature (at room temperature) θE = 440K. Our derived entropy Debye temperature (at 298 K) is θs = 320(± 3) K and the electron-phonon mass enhancement parameter is λ = 0.68." @default.
- W2059312069 created "2016-06-24" @default.
- W2059312069 creator A5055046311 @default.
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- W2059312069 date "1989-03-01" @default.
- W2059312069 modified "2023-10-02" @default.
- W2059312069 title "Thermodynamic properties of technetium" @default.
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- W2059312069 doi "https://doi.org/10.1016/0022-5088(89)90194-x" @default.
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