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• W2059481468 abstract "We performed a detailed low-energy electron-diffraction (LEED) analysis of (√7 × √7)R19.1°-S on Pd(111) and a re-analysis of (√3 × √3)R30°-S on Pd(111). Sulphur adsorption on the Pd(111) surface involves a (√3 × √3)R30° structure at room temperature, which by further exposure to H2S and heating to temperatures of approximately 450 K transforms irreversibly into a structure with (√7 × √7)R19.1° periodicity. There are distinct differences in the atomic structure of the high and the room temperature sulphur phases. For the (√3 × √3)R30° phase, we find the S atoms occupy fcc-hollow sites in agreement with a previous LEED analysis; we find, however, in contrast to the earlier analysis, adsorbate-induced relaxations of the Pd(111) surface. The present analysis permits one to reject all the simple sulphur overlayer geometries considered for the (√7 × √7)R19.1° structure and suggests that this phase comprises a mixed palladium-sulphur overlayer. However, a final conclusion regarding the exact atomic structure of this phase cannot yet be reached on the basis of the obtained level of agreement with the experimental LEED data." @default.
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• W2059481468 date "1994-09-01" @default.
• W2059481468 modified "2023-09-24" @default.
• W2059481468 title "Low-energy electron-diffraction analysis of the (√7 × √7)R19.1°-S adsorbate structure on the Pd(111) surface" @default.
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• W2059481468 doi "https://doi.org/10.1016/0039-6028(94)90255-0" @default.
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