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• W2059519985 abstract "The catalytic hydrolysis of urea was investigated under conditions relevant for the selective catalytic reduction of NOx (urea-SCR). The hydrolysis activities of the tested catalysts coated on cordierite monoliths were in the order ZrO2 > TiO2 > Al2O3 > H-ZSM-5 > SiO2. A comparison with isocyanic acid (HNCO) hydrolysis on the same catalysts showed that urea decomposition was much slower than HNCO hydrolysis; hence, catalytic urea thermolysis into NH3 and HNCO is likely to be the rate-determining step in urea decomposition. Interestingly, a different order of catalyst activities was found in water-free experiments on urea thermolysis: TiO2 > H-ZSM-5 ≈ Al2O3 > ZrO2 > SiO2. The widely accepted reaction pathway for urea decomposition, namely urea thermolysis followed by HNCO hydrolysis, seems to be valid on all the tested catalysts except ZrO2: The high urea hydrolysis activity of the ZrO2 catalyst compared to its low urea thermolysis activity suggested a different reaction pathway, in which water directly attacks adsorbed urea rather than adsorbed HNCO." @default.
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• W2059519985 date "2013-01-01" @default.
• W2059519985 modified "2023-09-26" @default.
• W2059519985 title "Catalytic urea hydrolysis in the selective catalytic reduction of NO_x: catalyst screening and kinetics on anatase TiO₂and ZrO₂" @default.
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• W2059519985 doi "https://doi.org/10.1039/c2cy20668d" @default.
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