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- W2059555637 abstract "Through the development of molecular beam experiments, quantum beats in isolated polyatomic molecules provide an interesting tool to obtain microscopic information. When collisions are unimportant, dephasing constants are neglected. The corresponding Fourier transform of the time-resolved signal is easily interpreted in simple terms of two resonances. However, if the collision processes become efficient or in condensed phase experiments, the dephasing constants must be accounted for. The author analyses the effects of pure dephasing on the Fourier spectrum in the experiments involving the study of quantum beats from polyatomic molecules. An exact analytical expression of the Fourier transform of the molecular density matrix is obtained. It is shown that the resonance linewidth increases almost linearly with the pure dephasing constant. Finally, the influence of the depopulation of the upper state is discussed." @default.
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- W2059555637 date "1983-10-28" @default.
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- W2059555637 title "Role of pure dephasing processes in molecular quantum beats" @default.
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- W2059555637 doi "https://doi.org/10.1088/0022-3700/16/20/014" @default.
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