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• W2059576380 abstract "Gold clusters and nanoparticles were deposited on the three kinds of porous coordination polymers (PCP5), MOF-5, CPL-2, and AI-MIL53 by the solid grinding method. The size of Au particles depended on the kinds of PCPs and increased in the order of AI-MIL53 < CPL-2 < MOF-5. The mean diameter of Au particles supported on AI-MIL53 was estimated to be 1.6 nm by HAADFSTEM. Such small Au clusters on AI-MIL53 can catalyze one-pot synthesis of secondary amines from primary amines by sequential oxidation/hydrogenation owing to the remarkable improvement of hydrogenation efficiency of imine. Gold clusters deposited on AI-MIL53 can also promoteN-alkylation of amine with alcohol to form a secondary amine under N2 atmosphere without using O2 and H2." @default.
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• W2059576380 date "2009-12-01" @default.
• W2059576380 modified "2023-10-16" @default.
• W2059576380 title "One-potN-alkylation of primary amines to secondary amines by gold clusters supported on porous coordination polymers" @default.
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• W2059576380 doi "https://doi.org/10.1007/bf03214948" @default.
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