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- W2059633340 abstract "The analysis of the pure rotational spectra of symmetric top molecules with unresolved K-structure is discussed. Expressions are derived giving the displacement of the observed peak maxima from the K = 0 lines using two approximations. The first, valid at large spectral slit widths, assumes that the observed maximum occurs at the center of gravity of the component K-lines. The second takes into account the effect of spectral slit width on the band contours. Both approximations yield rotational constants for NT3 which are in closer agreement with those obtained from rotation-vibration analyses than were the original far-infrared constants reported by McDowell and Jones, but the second approximation gives a much better statistical agreement. It is shown that when the second approximation is used, DJK can be obtained from far-infrared data even when the K-structure is not resolved. For NT3 the treatment yields DJK = −(12 ± 4) × 10−5cm−1, in good agreement with the theoretical value." @default.
- W2059633340 created "2016-06-24" @default.
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- W2059633340 date "1966-01-01" @default.
- W2059633340 modified "2023-09-23" @default.
- W2059633340 title "On the pure rotational spectra of symmetric top molecules with unresolved K-structure: Revision of the rotational constants of NT3" @default.
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- W2059633340 doi "https://doi.org/10.1016/0022-2852(66)90248-7" @default.
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