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- W2059796799 abstract "Abstract Fast radiationless deactivation S e ∼→ S 0 of a photoexcited state through a “funnel” is discussed. The experimental rates of such transitions cannot be explained in general by a one-dimensional model considering only the angle of isomerization. Inclusion of the full number of degrees of freedom leads to a multi-dimensional intersection of the adiabatic potential energy surfaces U e and U 0 in the region of the “funnel” where non-adiabatic interactions are strong and cause a fast electronic transition S e ∼→ S 0 . The rate constant of the isomerization reaction is found to be strongly related to the rate of rotational relaxation in the solvent and relaxation of the solvent orientational polarization." @default.
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- W2059796799 title "Photoisomerization through a “funnel” in polar and non-polar solvents" @default.
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- W2059796799 doi "https://doi.org/10.1016/0009-2614(85)80266-9" @default.
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