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- W2059862678 abstract "Theoretical predictions of the equilibrium elastic modulus of crosslinked amorphous polymers at low strain are compared. Different theories relate this modulus to the network structure, but are based on the different concepts of trapped entanglements, constrained junctions and constrained chains. To distinguish preferred theories, experimental conditions should be chosen to maximize differences of the predicted moduli. This is found to depend on choosing a polymer with high plateau modulus and either ideal end-linking or random crosslinking at a rather low level of random crosslinking (2 to 5 times that at the gel point). High initial values of Mn and Mw/Mn should be used, with no scission or dilution during crosslinking. Earlier tests of the theories were conducted under conditions where a ratio of the predicted moduli was less than 4. Experiments are proposed which would increase it to >20." @default.
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- W2059862678 date "1991-06-01" @default.
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- W2059862678 title "Effects of entanglements on elastic modulus of elastomer networks after terminal relaxation" @default.
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- W2059862678 doi "https://doi.org/10.1016/0022-3093(91)90699-7" @default.
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