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• W2060191423 abstract "Abstract Four group 12 metal halide/N‐donor organic ligand hybrid materials, ZnCl 2 (AEC) 2 ( 1 ), ZnI 2 (AEC) 2 ( 2 ), CdI 2 (AEC) 2 ( 3 ), and HgI 2 (AEC) 2 ( 4 ) [AEC=N‐(2‐aminoethyl)carbazole] were synthesized and characterized. Single crystals of ZnCl 2 (AEC) 2 · CH 3 CN ( 1· CH 3 CN) and ZnI 2 (AEC) 2 · CH 3 CN ( 2· CH 3 CN) were obtained from solutions. Single‐crystal X‐ray diffraction analysis revealed that 1· CH 3 CN and 2· CH 3 CN form quasi‐1D structures of (ZnCl 2 ) n and (ZnI 2 ) n chains. The two AEC ligands in one hybrid molecule are dissymmetric due to the steric hindrance effect of the AEC moiety and the hydrogen bonding of the CH 3 CN guest molecules. The UV/Vis spectra of compounds 1 – 4 were measured, and the optical energy gaps ( E g ) of compounds 1 – 3 are very close to that of AEC; the value of E g for compound 4 is a little smaller. Steady and transient photoluminescence studies revealed that the emissions of compounds 1 – 3 are attributed to the AEC ligands, whereas compound 4 does not emit light owing to the heavy‐atom effect. Theoretical studies of the electronic structures confirmed that the optical energy gaps and emissions of the hybrid materials are almost confined by the AEC organic ligand rather than the metal halides.(© Wiley‐VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2008)" @default.
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• W2060191423 date "2008-06-18" @default.
• W2060191423 modified "2023-09-22" @default.
• W2060191423 title "Metal Halide/N‐Donor Organic Ligand Hybrid Materials with Confined Energy Gaps and Emissions" @default.
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• W2060191423 doi "https://doi.org/10.1002/ejic.200800069" @default.
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