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- W2060398885 abstract "One of the most vexing problems in the liquid phase epitaxy of multiple-layer crystal structures is the control of layer thickness. Layer thickness are usually found to be much less than those calculated from liquidus data alone. Furthermore, the thickness of a given layer depends, in a complicated way, upon the growth times of previously-grown layers. By considering the kinetic limitations of slow solute diffusion through the solution to the growth interface, we have quantitatively explained this behavior and, by comparison to experiments by Dawson, Knight et al., and Bergh et al., have derived solute diffusion coefficients D for As in Ga, P in Ga, and rare-earth oxides in flux melts for bubble garnet. Over the temperature range 800 to 900 °C, D (As) follows an activation behavior: D (As) = 5000 exp (−20 000/T) and D (As, 800 °C) = 4.1 × 10−5 cm2/sec and D (As, 900 °C) = 1.8 × 10−4 cm2/sec. At 1020 °C, we find D (P) = 5.7 × 10−5 cm2/sec. For garnet flux melts at 846 °C, the rare-earth bearing species has a diffusion coefficient D = 5.8 (±1.3) × 10−7 cm2/sec. The present results show the complicated dependence of growth rate on time and degree of supersaturation. More importantly, one can now numerically simulate growth runs beforehand to rapidly and economically define experimental growth procedures." @default.
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- W2060398885 date "1973-08-01" @default.
- W2060398885 modified "2023-09-27" @default.
- W2060398885 title "Isothermal diffusion theory of LPE: GaAs, GaP, bubble garnet" @default.
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- W2060398885 doi "https://doi.org/10.1016/0022-0248(73)90031-6" @default.
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