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- W2060468082 abstract "Aqueous phase oxidation of SO2 or S(IV) by H2O2-metal ions at a H2O2 concentration much lower than S(IV), was studied using a continuously flowing stirred reactor. Of the metal ions, Fe2+ showed the highest catalytic activity, i.e. the oxidation of S(IV) continued after most of the H2O2 was consumed. The dependence of the rate on the concentration of S(IV), H2O2, Fe2+ or H+ and temperature was determined. The following rate expression and low apparent activation energy of 40.7 kJ mole−1 were evaluated,−d[S(IV)]/dt=620[S(IV)]2[Fe2+]0.5(molel−1S−1). The significance of this reaction as the sulfate formation in atmospheric water droplets is discussed and a comparison of the rate with others using H2O2, O3 and dissolved O2 catalyzed by metal ions is made." @default.
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- W2060468082 date "1990-01-01" @default.
- W2060468082 modified "2023-09-26" @default.
- W2060468082 title "Metal ion catalyzed oxidation of SO2 in the presence of trace H2O2 in aqueous solution under environmental reaction conditions" @default.
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- W2060468082 doi "https://doi.org/10.1016/0960-1686(90)90097-7" @default.
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