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- W2060542857 abstract "The isomerization of acetylene via hydrogen migration in intense laser fields (8 x 10(14) W/cm2) has been investigated by coincidence momentum imaging of the three-body Coulomb explosion process, C2H2 (3+)-->H+ + C+ + CH+. When ultrashort (9 fs) laser pulses are used, the angle between the momenta of C+ and H+ fragments exhibits a sharp distribution peaked at a small angle ( approximately 20 degrees ), showing that the hydrogen atom remains near the original carbon site in the acetylene configuration. On the other hand, a significantly broad distribution extending to larger momentum angles ( approximately 120 degrees ) is observed when the pulse duration is increased to 35 fs, indicating that the ultrafast isomerization to vinylidene is induced in the longer laser pulse." @default.
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- W2060542857 date "2008-02-25" @default.
- W2060542857 modified "2023-09-26" @default.
- W2060542857 title "Acetylene-vinylidene isomerization in ultrashort intense laser fields studied by triple ion-coincidence momentum imaging" @default.
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- W2060542857 doi "https://doi.org/10.1063/1.2828557" @default.
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