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- W2060698871 abstract "A facile solvothermal route is successfully developed to synthesize Bi4O5I2, a novel I-poor bismuth oxyiodide, with hierarchical nanoflake structure. The composition, structure, morphology, formation mechanism, photoabsorption, energy band, and photocatalytic properties of this material are systematically investigated. The results reveal that highly pure Bi4O5I2 can be easily obtained by reacting Bi3+, I−, and OH− at pH values of 6 to 10 under solvothermal conditions, and the formation of such hierarchical structure can be explained by a dissolution–recrystallization mechanism. The as-synthesized Bi4O5I2 nanoflakes show a favorable energy band structure (bandgap energy 2.17 eV, conduction band edge potential is more negative than the reduction potential of superoxide radicals), a high specific surface area (38.6 m2 g−1), and a hierarchical micro/nano structures. Thus, they exhibit superior photocatalytic and mineralization efficiency for the degradation of 4-tert-butylphenol (PTBP, a representative alkylphenol) under visible light irradiation, with a reaction rate is 6.8 and 57 times faster than that of BiOI microspheres and N-doped TiO2, respectively. The photogenerated reactive species and degradation intermediates are identified, and possible photocatalytic mechanism is proposed. What's more, the as-synthesized Bi4O5I2 nanoflakes remain stable during the photocatalytic reaction and can be used repeatedly, revealing their promising applications in the treatment of organic wastewaters." @default.
- W2060698871 created "2016-06-24" @default.
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- W2060698871 date "2014-04-01" @default.
- W2060698871 modified "2023-10-17" @default.
- W2060698871 title "Solvothermal synthesis of novel hierarchical Bi4O5I2 nanoflakes with highly visible light photocatalytic performance for the degradation of 4-tert-butylphenol" @default.
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- W2060698871 doi "https://doi.org/10.1016/j.apcatb.2013.10.055" @default.
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