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• W2060871258 abstract "Abstract Controlling the molecular structure of the donor–acceptor interface is essential to overcoming the efficiency bottleneck in organic photovoltaics. We present a study of self-assembled fullerene (C 60 ) molecular chains on perfectly ordered 6,13-dichloropentacene (DCP) monolayers forming on a vicinal Au(788) surface using scanning tunneling microscopy in conjunction with density functional theory calculations. DCP is a novel pentacene derivative optimized for photovoltaic applications. The molecules form a brick-wall patterned centered rectangular lattice with the long axis parallel to the monatomic steps that separate the 3.9 nm wide Au(111) terraces. The strong interaction between the C 60 molecules and the gold substrate is well screened by the DCP monolayer. At submonolayer C 60 coverage, the fullerene molecules form long parallel chains, 1.1 nm apart, with a rectangular arrangement instead of the expected close-packed configuration along the upper step edges. The perfectly ordered DCP structure is unaffected by the C 60 chain formation. The controlled sharp highly-ordered organic interface has the potential to improve the conversion efficiency in organic photovoltaics." @default.
• W2060871258 created "2016-06-24" @default.
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• W2060871258 date "2013-12-01" @default.
• W2060871258 modified "2023-09-27" @default.
• W2060871258 title "Sharp organic interface of molecular C60 chains and a pentacene derivative SAM on Au(788): A combined STM & DFT study" @default.
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• W2060871258 doi "https://doi.org/10.1016/j.susc.2013.08.015" @default.
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