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• W2061233620 endingPage "7906" @default.
• W2061233620 startingPage "7897" @default.
• W2061233620 abstract "Reactions of nickel (Ni−n, n=3–10), palladium (Pd−n, n=3–8), and platinum (Pt−n, n=3–7) cluster anions are investigated in a flow tube reactor. Rate coefficients are measured for reactions with N2, O2, CO2, and N2O. Reactions with O2, CO2, and N2O have rates that are greater than 10% of the collision rate for most clusters of four atoms or larger, while N2 reactions generally exhibit much lower reaction efficiencies. All the reactions studied show a strong dependence on cluster elemental composition. Many of the palladium cluster reactions are significantly faster than the corresponding nickel and platinum cluster reactions, while Ni−n and Pt−n have similar rate coefficients. Pt−6 is observed to have anomalously low rate constants for reactions with N2, CO2, and N2O compared to neighboring platinum clusters sizes and the nickel and palladium hexamers. N2, CO2, and O2 reactions are generally association reactions with varying degrees of cluster fragmentation observed. N2O reactions result in sequential addition of O atoms to the cluster. The extent of cluster fragmentation for the various reagents can be correlated with the estimated exothermicities of the adsorption processes." @default.
• W2061233620 created "2016-06-24" @default.
• W2061233620 creator A5051545854 @default.
• W2061233620 creator A5084566458 @default.
• W2061233620 date "1995-11-08" @default.
• W2061233620 modified "2023-10-18" @default.
• W2061233620 title "Chemisorption and oxidation reactions of nickel group cluster anions with N₂, O₂, CO₂, and N₂O" @default.
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• W2061233620 doi "https://doi.org/10.1063/1.470207" @default.
• W2061233620 hasPublicationYear "1995" @default.
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