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- W2061542227 abstract "Detection of nominal `zero kinetic energy electrons' in resonant two-photon ionization with (omega) 1 fixed and (omega) 2 scanned permits photoelectron spectroscopy with 1 - 5 cm -1 resolution. We report vibrational bands from 0 - 650 cm -1 for benzyl + -h 7 , benzyl + -(alpha) d 2 , and benzyl + -d 7 . The exocyclic C-C bond of benzyl cation has substantial double bond character. Band assignments from ab initio frequencies illuminate the mechanism of vibronic coupling in the 1 2 A 2 -2 2 B 2 system of neutral benzyl. In toluene + , we observe internal rotor frequencies that fix the V 6 barrier height of the CH 3 rotation at 20 +/- 5 cm -1 , which is remarkably low. In VO yields VO + + e - , we measure state-to-state relative photoionization cross sections from the intermediate spin-rotational state N' J' to different cation spin-rotation states N + J + . Remarkably strong lines corresponding to large changes in angular momentum ((Delta) N equals -6 to +7 and (Delta) J equals -6.5 to + 6.5) are observed. Accurate values of the adiabatic ionization potentials of each molecule are reported." @default.
- W2061542227 created "2016-06-24" @default.
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- W2061542227 date "1992-04-01" @default.
- W2061542227 modified "2023-09-23" @default.
- W2061542227 title "Photoelectron spectroscopy with cm-1resolution: VO+, benzyl+, toluene+" @default.
- W2061542227 doi "https://doi.org/10.1117/12.58157" @default.
- W2061542227 hasPublicationYear "1992" @default.
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