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- W2061763763 abstract "The influence of non-specific adsorption of reactants on the electrode impedance is discussed. A method is proposed for calculating the double layer parameters, starting from experimental values of q and Cd. Substitution of the double layer parameters in the expressions for the electrode impedance, derived by Delahay, makes it possible to predict the importance of non-specific adsorption. It appears that only for rather reversible electrode reactions (rate constant, ksh>0.1 cm s−1) adsorption effects can be expected. Theoretical predictions have been verified on the system Ba2+/Ba(Hg) in 0.1 and 1 M LiCl solutions. For both solutions no abnormal behaviour was found in the a.c. peak potential region, because the reaction is too irreversible (ksh=(9̄1)×10−3 cm s−1 and (1.6±0.3)×10−2 cm s−1 for resp. 1 M and 0.1 M LiCl solutions). The double layer capacity increases with Ba2+ concentration at potentials anodic of the a.c. peak, because of the non-specific Ba2+ adsorption." @default.
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- W2061763763 title "Influence of non-specific adsorption of reactants on the electrode impedance" @default.
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- W2061763763 doi "https://doi.org/10.1016/s0022-0728(70)80153-x" @default.
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