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• W2061781151 abstract "Pure rotational spectra of Ne–SH and Kr–SH have been studied by Fourier transform microwave spectroscopy. R-branch transitions in the lower-spin component (Ω=3/2) corresponding to a linear Πi2 radical were observed for J″=1.5–4.5 in the region 11–25 GHz for Ne–SH and for J″=1.5–6.5 in the region 5–20 GHz for Kr–SH, respectively, with parity doublings and hyperfine splittings associated with the H nucleus. Although the spectral pattern of Kr–SH is relatively regular, that of Ne–SH is irregular with the J dependence of the parity doublings quite different from other Rg–SH or Ar–OH complexes. Two-dimensional intermolecular potential energy surfaces (IPSs) for both of the species have been determined from the least-squares fittings of the observed rotational transitions utilizing results of high-level ab initio calculations. These IPSs reproduce the observed transition frequencies within the experimental error and provide accurate knowledge on the intermolecular interaction and internal dynamics. Systematic comparisons of Rg–SH complexes have clarified various features of this series of complexes." @default.
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• W2061781151 date "2004-03-30" @default.
• W2061781151 modified "2023-10-03" @default.
• W2061781151 title "Fourier transform microwave spectroscopy of the Rg–SH(2Πi) complexes (Rg:Ne, Kr): Determination of the intermolecular potential energy surfaces" @default.
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• W2061781151 doi "https://doi.org/10.1063/1.1669384" @default.
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