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- W2061916830 abstract "The unresolved issue of the maximum number of adsorbed ligands binding to SII Na+ cations contained in a Y zeolite has been investigated and explained using a new experimental approach, specially designed for the specific problem. The formation of Na+(CO)2 di-carbonyls has been identified for the first time for high CO coverage using a survey of IR spectra of the adsorbed CO. Also, the formation of Na+(CO)3 tri-carbonyls is confirmed and the conditions of its formation are thoroughly discussed. Moreover, the adsorption of the CO probe in the large NaY cavities is expressed in terms of four coexisting reactions reflecting the formation of the three Na–carbonyl species which involves the vacant coordination of sodium cations. This study refines the IR vibration bands of the three as-formed carbonyls of interest and provides new information towards the understanding at the molecular scale of how the three free coordination vacancies of Na+ sites sitting in SII positions can be investigated by means of CO binding." @default.
- W2061916830 created "2016-06-24" @default.
- W2061916830 creator A5084433942 @default.
- W2061916830 date "2010-01-01" @default.
- W2061916830 modified "2023-09-25" @default.
- W2061916830 title "Evidencing the three cationic coordination vacancies of SII Na+ in NaY zeolite: additional insights from IR surface species" @default.
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- W2061916830 doi "https://doi.org/10.1039/c0cp00276c" @default.
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