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- W2062214107 abstract "We have been developing tools for nonlinear spectroscopy aimed toward the ultimate goal of building a nonlinearspectrophotometer analogous to the ubiquitous linear spectrophotometer where a sample is placed in the instrument, abutton is pushed, and the absorption spectrum is obtained sometime later. This paper describes our progress toward thisgoal, describing many difficulties and complications as well as opportunities. We also show spectroscopic data andanalysis of a variety of materials that we have taken with preliminary nonlinear spectroscopic instrumentation we havealready developed. One of the more interesting observations obtained along this research path is the realization thatlinear dispersion theory can also be applied to nonlinear systems when formulated properly such that Kramers-Kronigrelations can be used to connect the dispersion of nonlinear refraction to the spectrum of nonlinear absorption. In somecircumstances this can be more easily applied to nonlinear systems than to linear systems since the nonlinear absorptionspectrum can be limited in wavelength. In addition, we have developed tools that can simultaneously give the spectrumof nonlinear absorption as well as the dispersion of the nonlinear refraction over an octave spectral range from 400nnmto 800 nm, the so called White-Light-Continuum Z-scan. Much of the research on nonlinear optical materials has been acollaborative effort requiring the skills and expertise of organic chemists and materials manufacturers. The goals of thispart of the research are to determine predictive structure-property relation capabilities. The database needed for thisresearch makes the nonlinear spectrophotometer a necessity." @default.
- W2062214107 created "2016-06-24" @default.
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- W2062214107 date "2009-10-07" @default.
- W2062214107 modified "2023-10-02" @default.
- W2062214107 title "Nonlinear spectroscopy: absorption and refraction" @default.
- W2062214107 doi "https://doi.org/10.1117/12.834788" @default.
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