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- W2062374520 abstract "Subsequent to our spectroscopic detection of the C2X(X=P,As) free radicals [F. X. Sunahori et al., J. Am. Chem. Soc. 129, 9600 (2007)], we have studied the electronic spectrum of the Δi2-X̃Πr2 system of the jet-cooled C2P free radical in the 490–630nm region. The high-resolution laser-induced fluorescence spectrum of the two spin components of the 000 band of C212P has been recorded, and the rotational and spin-orbit coupling constants have been determined for both electronic states. The Renner–Teller effect has been observed in both the Π2 and the Δ2 states, and the vibrational structure has been assigned. For the ground state, all of the observed levels up to 3500cm−1 were fitted with a standard Renner–Teller model. The excited Δ2 state vibrational levels were successfully fitted using literature energy level expressions derived from perturbation theory, yielding vibrational and Renner–Teller parameters for both C212P and C213P. The molecular structure of C2P in the ground and excited states has also been estimated and compared to ab initio calculations and the geometries of similar molecules." @default.
- W2062374520 created "2016-06-24" @default.
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- W2062374520 date "2008-06-27" @default.
- W2062374520 modified "2023-10-16" @default.
- W2062374520 title "The electronic spectrum of the C2P free radical and a Renner–Teller analysis of the Δ2 and X̃Π2 electronic states" @default.
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- W2062374520 doi "https://doi.org/10.1063/1.2939011" @default.
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