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- W2062479356 abstract "We calculate the electric-field-induced second-harmonic-generation (EFISH) susceptibility of a homogeneously broadened two-level system with permanent dipole moments. This susceptibility has contributions from the second-harmonic-generation (SHG) susceptibility of the same system without the presence of a dc field and the four-wave-mixing (FWM) component of the susceptibility ${ensuremath{gamma}}_{mathit{e}}$(-2ensuremath{omega};ensuremath{omega},ensuremath{omega},0). The magnitude and phase of the various contributions to EFISH arising from SHG and from FWM depend on the frequency of the fundamental optical field, the transition dipole moment ${mathrm{ensuremath{mu}}}_{mathit{a}mathit{b}}$, the permanent dipole moment of the ground-state level ${mathrm{ensuremath{mu}}}_{mathit{a}mathit{a}}$, and the difference of the ground- and excited-state dipole moments ensuremath{Delta}ensuremath{mu}. We present non-rotating-wave-approximation results for both the quasi-steady-state in systems where the dephasing time ${mathit{T}}_{2}$ is much shorter than the population decay time ${mathit{T}}_{1}$, so the polarization is in a steady state but the population is not, and for the complete steady state. Extraction of the SHG susceptibility from EFISH measurements is considered." @default.
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- W2062479356 date "1991-01-01" @default.
- W2062479356 modified "2023-10-14" @default.
- W2062479356 title "Relationship between second-harmonic generation and electric-field-induced second-harmonic generation" @default.
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- W2062479356 doi "https://doi.org/10.1103/physreva.43.507" @default.
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