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• W2062649334 abstract "Preparation of single-layer manganese oxide nanosheets (monosheets) comprised of edge-shared MnO6 octahedra has relied on multistep processing involving a high-temperature solid-state synthesis of bulk templates, and ion-exchange and exfoliation reactions in solutions, requiring high cost and long processing time. Here we demonstrate the first single-step approach to directly access the MnO2 monosheets, by the chemical oxidation of Mn2+ ions in the presence of tetramethylammonium cations in an aqueous solution. Of importance is that this template-free reaction readily proceeds within a day at room temperature. The ability of the MnO2 monosheets to self-assemble allows aggregation, to form layered structures with potassium cations and cationic tetrathiafulvalene analogues as intercalants. Furthermore, Langmuir−Blodgett (LB) films composed of the MnO2 monosheets were successfully fabricated by the LB deposition method, in which about one layer of the monosheets was deposited for each process." @default.
• W2062649334 created "2016-06-24" @default.
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• W2062649334 date "2008-11-01" @default.
• W2062649334 modified "2023-10-18" @default.
• W2062649334 title "Room-Temperature Synthesis of Manganese Oxide Monosheets" @default.
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• W2062649334 doi "https://doi.org/10.1021/ja804503f" @default.
• W2062649334 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18975943" @default.
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