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- W2062681085 abstract "Results of isobaric and isothermal studies of dielectric relaxation in a vitrifying orientationally disordered crystal ${[{(mathrm{C}{mathrm{H}}_{3})}_{3}mathrm{C}(mathrm{C}{mathrm{H}}_{2}mathrm{O}mathrm{H})]}_{0.70}{[{(mathrm{C}{mathrm{H}}_{3})}_{2}mathrm{C}{(mathrm{C}{mathrm{H}}_{2}mathrm{O}mathrm{H})}_{2}]}_{0.30}$ under pressures reaching $P=1.8phantom{rule{0.3em}{0ex}}mathrm{GPa}$ are discussed. The application of the linearized derivative-based analysis made it possible to detect validity domains of the Vogel-Fulcher-Tammann $ensuremath{tau}={ensuremath{tau}}_{0}^{mathit{VFT}}phantom{rule{0.2em}{0ex}}mathrm{exp}({D}_{T}{T}_{0}∕Tensuremath{-}{T}_{0})$ relation, the critical-like $ensuremath{tau}(T)ensuremath{propto}{(Tensuremath{-}{T}_{X})}^{ensuremath{-}g}$ dependence as well as their pressure counterparts. The agreement with predictions of the dynamical scaling model (DSM) is worth stressing. This suggests that the decoupling of translational and orientational degrees of freedom may be the key mechanism responsible for the validity of the DSM description for glassy systems. The application of high pressures led to the emergence of a phase transition, absent in studies under atmospheric pressure. The parametrization of the pressure evolution of the phase transition temperature $[{T}_{mathit{tr}}(P)]$ via the extended Simon-Glatzel-type relation suggests the possible maximum of ${T}_{mathit{tr}}(P)$ at extreme pressures. It is concluded that the nontypical increase of the fragility strength coefficient $({D}_{T})$ noted on cooling in studies under atmospheric pressure [A. Drozd-Rzoska et al., Phys. Rev. B 73, 224205 (2006)] may be due to approaching the phase transition hidden under compression." @default.
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- W2062681085 date "2006-08-02" @default.
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- W2062681085 title "Dielectric relaxation in compressed glassy and orientationally disordered mixed crystals" @default.
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- W2062681085 doi "https://doi.org/10.1103/physrevb.74.064201" @default.
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