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• W2062743156 abstract "Catalytic combustion is a practical approach to sustain and manage combustion in microreactors. Previous work has demonstrated room-temperature ignition and size-dependent properties of platinum nanoparticles as they related to catalytic combustion of hydrocarbons. This work investigates the use of platinum nanoparticle coatings to combust a stochiometric methanol–air mixture. Platinum nanoparticles with dp = 8 nm were used to coat cordierite substrates with 800 μm wide square channels. Room-temperature ignition of the methanol–air mixture and repeated catalytic cycling were successfully achieved with operational temperatures ranging from 250 to 850 °C. The catalysis reaction was controlled by altering fuel–air flow rates and catalyst mass loading. A nanoparticle stability study indicated a minimal effect of sintering on the combustion behavior and vice versa with repeated catalytic cycling. A product gas analysis indicated that overall methanol conversion rates of up to 60% were achieved with the current design. The results of this work directly contribute to the development of catalytic micrometer-scale combustors." @default.
• W2062743156 created "2016-06-24" @default.
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• W2062743156 date "2013-07-02" @default.
• W2062743156 modified "2023-10-16" @default.
• W2062743156 title "Platinum-Nanoparticle-Catalyzed Combustion of a Methanol–Air Mixture" @default.
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• W2062743156 doi "https://doi.org/10.1021/ef400424e" @default.
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