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- W2062751072 abstract "A theory of the electron-transfer reaction at the boundary between an electrode and an electrolytic solution is discussed as a heterogeneous process, in analogy with the metal-rectifier theory, according to the contact model proposed in the previous paper. Using the theory of the absolute reaction rate, the rate constant is related to the partition function of the substances participating in this reaction. The relation between the faradaic current and the applied polarization, i.e., the so-called overpotential, can be theoretically derived in a similar form with the familiar expression. Various kinetic parameters, e.g., α value, rate constant etc., may be exactly rearranged as a problem of statistical mechanics and electromagnetism." @default.
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- W2062751072 date "1967-06-15" @default.
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- W2062751072 title "Theoretical Model for Metal Electrode in Electrolytic Solution. II. Absolute Rate Theory of Heterogeneous Electron‐Transfer Reaction" @default.
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- W2062751072 doi "https://doi.org/10.1063/1.1840614" @default.
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