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• W2062831285 abstract "Formation of 1:1, 1:2, and 1:3 binary complexes of Th(IV), UO2(II), Ce(III), and La(III) metal ions with acetohydroxamic acid (Aha), benzohydroxamic acid (Bha), and salicylhydroxamic acid (Sham) was investigated in aqueous medium using the potentiometric technique at 25 °C and I = 0.10 mol·dm-3 NaNO3. The order of stability of the complexes was investigated and is discussed in terms of both the nature of hydroxamic acid and the metal ion. The concentration distribution of various species formed in solution was evaluated. Evaluation of the effect of temperature of the medium on the ionization process of ligands and the stability of 1:1 binary complexes has been performed at I = 0.10 mol·dm-3 NaNO3, and the corresponding thermodynamic parameters have been calculated and are discussed as well. Evaluation of the effect of ionic strength of the medium on both the dissociation process and the stability of metal complexes for Sham binary systems is reported. In addition, the dissociation constants of Aha and stability constants of its 1:1 binary complexes were determined in various water + dioxane mixtures under the experimental conditions (t = 25 °C, I = 0.10 mol·dm-3 NaNO3). It was concluded that solvent effects have a profound influence on the proton−ligand and metal−ligand stability constants. Confirmation of the formation of binary complexes in solution has been done using conductivity, cyclic voltammetry, and UV−visible spectroscopic measurements." @default.
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• W2062831285 date "2007-08-24" @default.
• W2062831285 modified "2023-10-15" @default.
• W2062831285 title "Equilibrium Studies of Binary Systems Involving Lanthanide and Actinide Metal Ions and Some Selected Aliphatic and Aromatic Monohydroxamic Acids" @default.
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• W2062831285 doi "https://doi.org/10.1021/je600541a" @default.
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