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- W2062844410 abstract "Abstract Recent experiments on gaseous iodine and β‐carotene are analyzed within a wave‐packet description of femtosecond‐time resolved four‐wave mixing spectroscopy. Employing the same formalism, two different experimental setups, both established in the Kiefer group, are treated. In a transient four‐wave‐mixing (FWM) experiment, where two pulses interact simultaneously with the system, the interaction with a third time‐delayed pulse leads to light emission reflecting ground state vibrational dynamics in I 2 . On the other hand, delaying a FWM‐pulse sequence with respect to a single pump pulse interacting with β‐carotene yields a signal that is directly proportional to the population of a selected nuclear eigenstate in the electronic ground state. Thus, within this setup, it is possible to monitor ground‐state re‐population dynamics mode specifically. Copyright © 2006 John Wiley & Sons, Ltd." @default.
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- W2062844410 date "2006-01-01" @default.
- W2062844410 modified "2023-09-27" @default.
- W2062844410 title "Ground state vibrational wave-packet and recovery dynamics studied by time-resolved CARS and pump-CARS spectroscopy" @default.
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- W2062844410 doi "https://doi.org/10.1002/jrs.1441" @default.
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