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• W2063005247 abstract "Achiral molecules of 5,5‘,6,6‘-tetrachlorobenzimidacarbocyanine dyes having 1,1‘-di-n-alkyl substituents longer than hexyl combined with 3,3‘-bis(2-acidoethyl) or 3,3‘-bis(3-acido-n-propyl) substituents form J-aggregates whose absorption spectrum exhibits Davydov-split subbands that display strong circular dichroism, indicating the enantioselective formation of chiral J-aggregates. In this way, for the first time, in the liquid phase self-organization of achiral dye molecules to chiral supramolecular aggregates has been realized which can be controlled by the molecular structure of the monomeric precursors. A helix-like, cylindric structure of the chiral J-aggregates is suggested. The results expose an interesting model for studying and understanding enantioselective processes in the biosphere." @default.
• W2063005247 created "2016-06-24" @default.
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• W2063005247 date "1997-07-01" @default.
• W2063005247 modified "2023-09-27" @default.
• W2063005247 title "Structural Conditions for Spontaneous Generation of Optical Activity in J-Aggregates" @default.
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• W2063005247 doi "https://doi.org/10.1021/jp9708308" @default.
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