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- W2063011043 abstract "Waves moving over the surface of a Rh field emitter tip in an oscillatory way during the NO-H2 reaction have been visualized earlier by field electron microscopy (FEM). An autocatalysis model has been proposed to describe the oscillatory behaviour of the reduction of NO by H2. To study the oscillatory behaviour and the effect of the surface structure in more detail a large Rh(100) surface and a large stepped Rh(533) surface, Rh[4(111)∗(100)], have been selected. The first results show that, in correspondence with the FEM experiments, rate oscillations could be observed over the Rh(533) surface in the 10−6 mbar pressure regime around 470 K. No oscillatory behaviour was obtained on the Rh(100) surface under these conditions. The structure-sensitivity of the process is related to the large dependence of the Rh-N bond strength on the surface structure. Nitrogen desorbs at a much higher temperature from Rh(100) than from Rh(533)." @default.
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- W2063011043 date "1994-11-01" @default.
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- W2063011043 title "Oscillatory behaviour of the NOH2 reaction over Rh(533)" @default.
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- W2063011043 doi "https://doi.org/10.1016/0039-6028(94)90586-x" @default.
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