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• W2063143678 startingPage "4739" @default.
• W2063143678 abstract "Eleven commercial stabilized and unstabilized zirconia and titania samples have been tested for stability as potential catalyst supports for supercritical water gasification at 400 °C and 28.5 MPa. Samples based on monoclinic zirconia and rutile as well as one sample based on stabilized tetragonal zirconia showed good physical stability. Most samples showed a loss of surface area during the first 20 h of hydrothermal treatment, leveling out at longer exposure times. In a continuous fixed-bed reactor setup, a performance and stability test of the samples loaded with 2 wt % ruthenium gave good results for three samples, of which the sample based on stabilized tetragonal zirconia showed the best performance. For those samples, the surface area decreased only to a minor extent, which we attribute to an aging step that has been performed prior to impregnation with ruthenium. The metal surface area showed a minor decrease for all samples. The reason for this decrease is probably the build-up of a layer of carbon deposit on top of the active sites." @default.
• W2063143678 created "2016-06-24" @default.
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• W2063143678 date "2013-07-24" @default.
• W2063143678 modified "2023-09-24" @default.
• W2063143678 title "Stability and Performance of Ruthenium Catalysts Based on Refractory Oxide Supports in Supercritical Water Conditions" @default.
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• W2063143678 doi "https://doi.org/10.1021/ef400707f" @default.
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