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- W2063189391 abstract "A new synthetic strategy for heterocyclic compounds with transition metal-catalyzed reaction was developed. It was demonstrated that carbonyl moiety in a cyclic compound is susceptible to nucleophilic attack of nickel(0) complex, which allows an intermolecular formal [4+2] cycloaddition to alkynes via decarbonylation, decaroxylation or elimination of ketone. A nickel-catalyzed decarbonylative cycloadditon of N-arylphthalimides with alkynes affords substituted isoquinolones. A decarbonylative cycloaddition of phthalic anhydrides to alkynes is also successfully demonstrated using a nickel catalyst in association with a Lewis acid as a co-catalyst. A carboamination of alkynes with isatoic anhydrides to form quinolones is also achieved by a nickel-catalyzed decarboxylative cycloaddition. It is also demonstrated that a cycloaddition of salicylic acid ketal to alkyne using a nickel catalyst forms chromones through an elimination of a ketone." @default.
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- W2063189391 date "2010-01-01" @default.
- W2063189391 modified "2023-09-23" @default.
- W2063189391 title "Syntheses of Heterocycles by Nickel-catalyzed Substitution Reaction" @default.
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- W2063189391 doi "https://doi.org/10.5059/yukigoseikyokaishi.68.33" @default.
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