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• W2063287029 abstract "Abstract The entropies of melting of LiNO 2 , NaNO 2 , KNO 2 , RbNO 2 , CsNO 2 , and TlNO 2 , have been determined by DSC. For KNO 2 , RbNO 2 , CsNO 2 , and TlNO 2 , they are much smaller than those of the corresponding alkali chlorides. The small entropy values are compensated for by the large entropies of the transitions that occur at lower temperatures. For LiNO 2 , no phase transition takes place below the melting temperature. NaNO 2 undergoes a solid-solid phase transition associated with a small entropy change. The sum of the entropies of melting and transitions (if there are any) is approximately constant (40 J K −1 mol −1 ) for all of the nitrites studied. Plastic flow of the high-temperature phase of TlNO 2 under stress was measured and found to be comparable in magnitude with that of typical organic plastic crystals. Literature values of Δ m S and Δ trs S of 19 A + B − -type ionic crystals were surveyed. It was found that values of Δ m S are smaller than those of the corresponding alkali chlorides. The extension of the classification of the plastically crystalline state in the original molecular crystals to the ionic crystal is proposed. In contrast to the accepted view that the weak intermolecular forces in molecular crystals favor formation of plastic phases, an argument is put forward that the strong Coulombic attraction stabilizes the plastically crystalline phase of the ionic crystals by holding together the orientationally disordered molecular ions." @default.
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• W2063287029 date "1988-09-01" @default.
• W2063287029 modified "2023-09-24" @default.
• W2063287029 title "Thermodynamic properties of alkali and thallium nitrites: the ionic plastically crystalline state" @default.
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• W2063287029 doi "https://doi.org/10.1016/0040-6031(88)87103-x" @default.
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